Stability of (3)He(2)(4)He(n) and (3)He(3)(4)He(n) L=0 clusters.

نویسندگان

  • Dario Bressanini
  • Gabriele Morosi
چکیده

We have studied the stability of mixed (3)He/(4)He clusters in L=0 states by the diffusion Monte Carlo method, employing the Tang-Toennies-Yiu He-He potential. The clusters (3)He(4)He(N) and (3)He(2)(4)He(N) are stable for N>1. The lighter atoms tend to move to the surface of the cluster. The minimum number of 4He atoms able to bind three 3He atoms in a L=0 state is nine. Two of three fermionic helium atoms stay on the surface, while the third one penetrates into the cluster.

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Microsolvation of NO2+ in Helium: An Ab Initio Study on NO2+-Hen Clusters (n ≤ 7)

      In this study, the interaction between NO2+ cation and Hen (n = 1-7) clusters is investigated by means of ab initio calculations at MP2/aug-cc-pVTZ and QCISD/aug-cc-pVTZ computational levels. The first and second solvation shells were obtained while N atom of NO2+ interacts with five and two He atoms, respectively. Stabilizat...

متن کامل

ar X iv : c on d - m at / 0 30 35 00 v 1 2 4 M ar 2 00 3 From nonwetting to prewetting : the asymptotic behavior of 4 He drops on alkali substrates

We investigate the spreading of 4 He droplets on alkali surfaces at zero temperature, within the frame of Finite Range Density Functional theory. The equilibrium configurations of several 4 He N clusters and their asymptotic trend with increasing particle number N , which can be traced to the wetting behavior of the quantum fluid, are examined for nanoscopic droplets. We discuss the size effect...

متن کامل

Solvent states and spectroscopy of doped helium clusters as a quantum-chemistry-like problem.

The Full-Configuration-Interaction Nuclear-Orbital (FCI-NO) approach [J. Chem. Phys., 2009, 131, 19401], as the implementation of the quantum-chemistry ansatz, is overviewed and applied to (He)N-Cl2(X) clusters (N≤ 4). The ground and excited states of both fermionic (3)He and bosonic (4)He [see also, J. Phys. Chem. Lett., 2012, 2, 2145] clusters are studied. It is shown that the FCI-NO approach...

متن کامل

X iv : n uc l - ex / 9 60 70 11 v 1 1 9 Ju l 1 99 6 Measurements of the Total Cross Section for the Scattering of Polarized Neutrons from Polarized 3 He

Measurements of polarized neutron—polarized 3 He scattering are reported. The target consisted of cryogenically-polarized solid 3 He, thickness 0.04 atom/b and polarization ∼ 0.4. Polarized neutrons were produced via the 3 H(p, n) 3 He or 2 H(d, n) 3 He polarization-transfer reactions. The longitudinal and transverse total cross-section differences ∆σ L and ∆σ T were measured for incident neutr...

متن کامل

On Associated and Generalized Lah Numbers and Applications to Discrete Distributions

Bin, r, k) = 0 fo r k > n, B(n9 r9 0) = 0 , Bin, r, 1) = r(r + l ) . . . ( p + n 1 ) , Bin, v, ri) = v and Bin, ls k) = \L(n9 k) | , t h e s i g n l e s s Lah numbers ( see Riordan [ 1 2 ] , p . 4 4 ) . Ahuja & Enneking have a l s o ob ta ined (see [2]) t he fo l lowing r e l a t i o n s for t he B(n9 r9 k)'s: Bin + 1, v9 k) = in + rk)B(n9 v9 k) + vBin, r, k 1 ) , (2) and [Bin9 v9 k)] > Bin, v,...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

عنوان ژورنال:
  • Physical review letters

دوره 90 13  شماره 

صفحات  -

تاریخ انتشار 2003